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21.
Trends of perfluorochemicals in Greenland ringed seals and polar bears: Indications of shifts to decreasing trends 总被引:1,自引:0,他引:1
Time-series of perfluorinated alkylated substances (PFASs) in East Greenland polar bears and East and West Greenland ringed seals were updated in order to deduce whether a response to the major reduction in perfluoroalkyl production in the early 2000s had occurred. Previous studies had documented an exponential increase of perfluorooctane sulphonate (PFOS) in liver tissue from both species. In the present study, PFOS was still the far most dominant compound constituting 92% (West Greenland ringed seals), 88% (East Greenland ringed seals) and 85% (East Greenland polar bears). The PFOS concentrations increased up to 2006 with doubling times of approximately 6 years for the ringed seal populations and 14 years in case of polar bears. Since then a rapid decrease has occurred with clearing half-lives of approximately 1, 2 and 4 years, respectively. In polar bears perfluorohexane sulphonate (PFHxS) and perfluorooctane sulphonamide (PFOSA) also showed decreasing trends in recent years as do perfluorodecanoic acid (PFDA) and perfluoroundecanoic acid (PFUnA). For the West Greenland ringed seal population perfluorooctanoic acid (PFOA), perfluorononanoic acid (PFNA), PFDA and PFUnA peaked in the mid 2000s, whereas PFNA, PFDA and PFUnA in the East Greenland population have been stable or increasing in recent years. The peak of PFASs in Greenland ringed seals and polar bears occurred at a later time than in Canadian seals and polar bears and considerably later than observed in seal species from more southern latitudes. We suggest that this could be explained by the distance to emission hot-spots and differences in long-range transport to the Arctic. 相似文献
22.
Pavel Karásek Barbora Hohnová Josef Planeta Lenka Št’avíková Michal Roth 《Chemosphere》2013,90(6):2035-2040
Increasing production and disposal of organic light-emitting diode (OLED) displays for smartphones and tablets may have impact on the environment depending on the aqueous solubility of the pertinent chemicals. Here, aqueous solubilities are presented for several compounds, mostly aromatic amines, used as hole transport materials in the OLED displays. Solute selection includes 1,4-bis(diphenylamino)benzene, tetra-N-phenylbenzidine, 4,4′-bis(N-carbazolyl)-1,1′-biphenyl, 1,3,5-tris(diphenylamino)benzene, and 9,10-bis(phenylethynyl)anthracene. The solubilities are those in pressurized hot water (PHW), i.e., measured at elevated temperature (up to 260 °C) and pressure. The semi-quantitative estimates of room-temperature solubilities of the solutes have been obtained from extrapolations of the solubilities in PHW. For the compounds studied, the estimated aqueous solubilities at room temperature do not exceed 2 × 10?11 g of the solute per 1 kg of water. Aqueous solubilities of triphenylamine have also been measured and used to upgrade a recent group-contribution model of aqueous solubilities of organic nonelectrolytes with the parameters for the nitrogen atom in aromatic amines. 相似文献
23.
Bilodeau Gauthier S Houle D Gagnon C Côté B Messier C 《Journal of environmental quality》2008,37(3):871-879
Dendrochemistry has been used for the historical dating of pollution. Its reliability is questionable due primarily to the radial mobility of elements in sapwood. In the present study, the extractability of seven elements was characterized to assess their suitability for the monitoring of environmental conditions. Nine mature sugar maple trees (Acer saccharum Marsh.), a wide-ranging species in eastern North America that has suffered decline in past decades, were sampled in three Quebec watersheds along a soil acidity gradient. Five-year groups of annual tree rings were treated by sequential chemical extractions using extractants of varying strength (deionized H2O, 0.05 M HCl, and concentrated HNO(3)) to selectively solubilize the elements into three fractions (water-soluble, acid-soluble, and residual). Monovalent K; divalent Ba, Ca, Cd, Mg, Mn; and trivalent Al cations were found mostly in the water-soluble, acid-soluble, and residual fractions, respectively. Forms more likely to be mobile within the tree (water-soluble and acid-soluble) do not seem to be suitable for temporal monitoring because of potential lateral redistribution in sapwood rings. However, certain elements (Cd, Mn) were responsive to current soil acidity and could be used in spatial variation monitoring. Extractability of Al varied according to soil acidity; at less acidic sites, up to 90% of Al was contained in the residual form, whereas on very acidic soils, as much as 45% was found in the water-soluble and acid-soluble fractions. Sequential extractions can be useful for determining specific forms of metals as key indicators of soil acidification. 相似文献
24.
This paper introduces an integrated water management model at the industrial park level. It suggests four approaches to water
management: first, direct water reuse among users; second, water reuse among users by blending with freshwater; third, water
reuse between users and a wastewater treatment plant; and fourth, groundwater recharge by reclaimed wastewater or other feasible
applications in order to optimize the overall water efficiency. The model results in a comprehensive management methodology
for optimizing water resources within an industrial park, seeking potential water reuse among industries, and incorporating
the size and cost of reclaimed wastewater delivery systems. A case study is employed to test the model’s feasibility. An economic
analysis of the optimized water use network is also carried out, showing the potential water and cost savings. 相似文献
25.
26.
Sonia Rombout Daniel Sartenaer Benoît Parmentier Christian Dugauquier Yves Gillerot 《黑龙江环境通报》2004,24(10):822-827
We present a case of de novo trisomy of distal 19q diagnosed prenatally by cytogenetics and FISH analysis. The autopsy performed after termination of the pregnancy showed major internal and external malformations that are associated with this chromosome abnormality. Copyright © 2004 John Wiley & Sons, Ltd. 相似文献
27.
Petrash Daniel A. Novák Martin Bohdálková Leona Krachler Micheal Čuřík Jan Veselovský František Štěpánová Markéta Umbría-Salinas Karelys Přechová Eva Komárek Arnost 《Environmental science and pollution research international》2021,28(13):16107-16121
Environmental Science and Pollution Research - Arsenic (As) concentrations and deposition fluxes were measured in snow and rime at 10 mountain-top sites near the borders between the Czech Republic... 相似文献
28.
Kinga Kostrakiewicz-Gierałt 《Russian Journal of Ecology》2018,49(1):47-52
The impact of succession stage on the share of clonal plants in the plant cover, seed rain and seedling pool has been studied in the years 2014 and 2015. The investigations were carried out in abandoned Molinion caeruleae meadows dominated by small-statured species (Patch I), tall growing large-tussock grasses (Patch II) and shrub-willows (Patch III). Although the clonal taxa dominated in the plant cover, seed rain and seedling pool, their share in subsequent study sites was quite different. The spectra of life-history traits relevant to clonality in the plant cover and seed rain were similar and did not vary significantly among subsequent locations, while they mostly differed as observed in the seedling pool. The various spectra observed in seedling pool in subsequent study sites might be due to fact that the seed germination and recruitment of offspring are strongly influenced by habitat conditions which varied remarkably in the successive Patches. 相似文献
29.
Cuyler Christine Rowell Janice Adamczewski Jan Anderson Morgan Blake John Bretten Tord Brodeur Vincent Campbell Mitch Checkley Sylvia L. Cluff H. Dean Côté Steeve D. Davison Tracy Dumond Mathieu Ford Barrie Gruzdev Alexander Gunn Anne Jones Patrick Kutz Susan Leclerc Lisa-Marie Mallory Conor Mavrot Fabien Mosbacher Jesper Bruun Okhlopkov Innokentiy Mikhailovich Reynolds Patricia Schmidt Niels Martin Sipko Taras Suitor Mike Tomaselli Matilde Ytrehus Bjørnar 《Ambio》2020,49(3):805-819
Ambio - Muskoxen (Ovibos moschatus) are an integral component of Arctic biodiversity. Given low genetic diversity, their ability to respond to future and rapid Arctic change is unknown, although... 相似文献
30.
Environmental Monitoring and Assessment - The present study aims to estimate the effects of PM2.5 on the health and economy of Karaj city from 2012 to 2019. In this study, mortality attributed to... 相似文献